Oxidation-Induced Changes in the Lattice Structure of YSZ Deposited by EB-PVD in High-Vacuum Conditions

Author:

Lee Gye-Won12,Lee In-Hwan2ORCID,Oh Yoon-Suk1

Affiliation:

1. Engineering Materials Center, Korea Institute of Ceramic Engineering and Technology, Icheon 17303, Republic of Korea

2. Department of Materials Science and Engineering, Korea University, 145 Anam-ro, Seongbuk-gu, Seoul 02841, Republic of Korea

Abstract

Yttria-stabilized zirconia (YSZ), a thermal barrier coating material characterized by low thermal conductivity, is typically deposited via electron beam-physical vapor deposition. Notably, oxygen depletion occurs during this process, causing color changes in YSZ. Therefore, YSZ is speculated to undergo phase transformation during this process, which demands careful consideration owing to its effect on the life of thermal coatings. To study this phenomenon, bulk samples were prepared, subjected to vacuum heat treatment to induce oxygen depletion, and followed by oxidative heat treatment. Experimental results showed that the color of the samples changed to black after the vacuum heat treatment and to a lighter color after the oxidative heat treatment. In addition, X-ray diffraction and Raman analyses were performed. The monoclinic phase formation was confirmed during the vacuum heat treatment; however, it disappeared after the oxidation heat treatment. The coating obtained in a high vacuum atmosphere exhibited a black color and cubic phase, which changed to a bright color and tetragonal phase after the oxidation heat treatment.

Funder

Institute of Civil Military Technology Cooperation, Civil-Military Technology Development

Publisher

MDPI AG

Subject

Process Chemistry and Technology,Chemical Engineering (miscellaneous),Bioengineering

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