The Preparation of Mn-Modified CeO2 Nanosphere Catalysts and Their Catalytic Performance for Soot Combustion

Author:

Gao Siyu1,Yu Di2,Zhou Shengran1,Zhang Chunlei1,Wang Lanyi2,Fan Xiaoqiang1,Yu Xuehua1ORCID,Zhao Zhen12

Affiliation:

1. Institute of Catalysis for Energy and Environment, College of Chemistry and Chemical Engineering, Shenyang Normal University, 253# Huanghe North Street, Huanggu District, Shenyang 110034, China

2. State Key Laboratory of Heavy Oil Processing, China University of Petroleum, 18#Fuxue Road, Chang Ping, Beijing 102249, China

Abstract

With the increasing stringency of environmental protection regulations, reducing the severe pollution caused by soot particles from diesel vehicle exhaust has become a widespread concern. Catalytic purification technology is currently an efficient method for eliminating soot particles, which needs to develop high-activity catalysts. This work uses a two-step hydrothermal method to synthesize MnOx/CeO2 nanosphere catalysts, which have synergistic effects between manganese and cerium, and have high reactive oxygen species. Among them, the MnCe-1:4 catalyst represents the optimal catalytic activity, and the values of T10, T50, and T90 are 289, 340, and 373 °C, respectively. On account of their simple synthetic procedure and low cost, the prepared MnOx/CeO2 nanosphere catalysts have good prospects for practical applications.

Funder

National Key R&D Program of China

National Natural Science Foundation of China

Excellent Youth Science Foundation of Liaoning Province

Shenyang Science and Technology Planning Project

University Joint Education Project for China-Central and Eastern European Countries

Major/Key Project of Graduate Education and Teaching Reform of Shenyang Normal University

Publisher

MDPI AG

Subject

Process Chemistry and Technology,Chemical Engineering (miscellaneous),Bioengineering

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