Input Flux and the Risk of Heavy Metal(Loid) of Agricultural Soil in China: Based on Spatiotemporal Heterogeneity from 2000 to 2021

Abstract

Identifying the current status of the heavy metal(loid) input of agricultural soils is vital for the soil ecological environment of agricultural-producing areas. Most previous studies have typically carried been out in small regions with limited sampling sites, which is insufficient to reveal the overall status of China. This study reviewed publications from over the past 20 years and calculated the input fluxes of heavy metal(loid)s in agricultural soil via atmospheric deposition, fertilizer, manure, and irrigation in different regions of China based on spatiotemporal heterogeneity using a meta-analysis, providing more accurate and reliable results. It was found that the heavy metal(loid) input flux of atmospheric deposition in China is large, while that of fertilizer and manure is relatively low compared to Europe. The major sources of As, Cd, Cr, Ni, and Pb entering the soil was atmospheric deposition, which accounted for 12% to 92% of the total input. Manure was responsible for 19% to 75% of the Cu and Zn input. Cd is the element presenting the most significant risk to the environment of agricultural soils in China and its safety limit will be reached within 100 years for most regions. The region we need to be concerned about is Huang-Huai-Hai due to its comprehensive pollution.