Development and Characterization of a Time-Sequenced Cascade Impactor: Application to Transient PM2.5 Pollution Events in Urbanized and Industrialized Environments

Author:

Ngagine Soulemane HalifORCID,Deboudt KarineORCID,Flament PascalORCID,Choël MarieORCID,Kulinski Pierre,Marteel Fabien

Abstract

To set up a sampling and analysis strategy for particulate matter (PM) based on the time periods used in international standards is often inadequate for assessing the impact of day/night cycles or episodic emissions on urban air quality. To obtain a detailed physico–chemical characterization of urban PM when concentrations exceed the regulatory thresholds, a new rotary cascade impactor named the Time-Resolved Atmospheric Particle Sampler (TRAPS) was designed and tested for coarse and fine particle sampling. The TRAPS implementation, coupled with Optical Particle Counter measurements, provides time-resolved samples that can be analyzed by a wide range of single-particle analysis techniques. The TRAPS theoretical design was verified experimentally. Experimental cut-off diameters of 1.32 and 0.13 µm, respectively, for coarse and fine stages, were found in good agreement with theoretical values. Additionally, good trace separation, preventing inter-sample contamination, was evidenced by Scanning Electron Microscopy (SEM). The homogeneous distribution of particles of different types over a trace was also verified. As a case study, automated SEM-EDX analysis of 2500 particles, collected during two pollution peaks of a transient PM2.5 pollution event, revealed that individual particles’ chemical composition was influenced by local sources during the first pollution peak, and mainly transported during the second peak.

Funder

Agence Nationale de la Recherche

Publisher

MDPI AG

Subject

Atmospheric Science,Environmental Science (miscellaneous)

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