Temporal and Spatial Modal Analysis and Prediction of Tropospheric CO Concentration over the World and East Asia

Abstract

Spatiotemporal modal analysis and prediction of tropospheric atmospheric CO concentration in the world and East Asia from 2002 to 2021 using the inversion data of airs sounder. The results show that: The CO concentration in the northern hemisphere is higher than that in the southern hemisphere; from the upper troposphere to the lower troposphere, the CO concentration changes from “∧“ to “√”; the fluctuation range of near surface CO concentration in the northern hemisphere is relatively intense, and the fluctuation range in the southern hemisphere is relatively small. Using MK, Sen slope estimation, and EOF analysis, it is found that CO concentration in the convective middle layer tends to decline in more than 90% of the global area, and the decline rate in the northern hemisphere is significantly higher than that in the southern hemisphere. In East Asia, the CO concentration in the lower tropospheric marine area is significantly lower than that in the land area. The average concentration and decline rate of CO in East Asia is always higher than that in the world; the CO concentration in East Asia is the highest in spring and winter in the lower troposphere; and the CO concentration in East Asia is lower in the northeast and higher in the southeast in the upper troposphere in spring, autumn, and winter, and higher in the northeast and Central Plains in summer. Compared with the three-exponential smoothing model, the prediction error of the VMD-LSTM hybrid model for atmospheric CO concentration is significantly reduced, which indicates that the improved neural network prediction model has higher prediction accuracy. The factors affecting the change of tropospheric CO concentration are not only affected by the ground factors, but also related to indirect factors such as water vapor, methane, and atmospheric temperature in the atmosphere.