3D Imaging of On-Chip Porous Medium Using X-ray Laminography: Application to Reactive Flow Dissolution at Small Scales

Author:

Morais Sandy1,Lecoutre Carole1ORCID,Philippot Gilles1ORCID,Aubert Guillaume1ORCID,Nguyen Olivier1,Cario Anaïs1,Vidal Emeline1,Campbell Zachary S.2,Garrabos Yves1,Azaroual Mohamed3ORCID,Helfen Lukas45,Bernard Dominique1,Marre Samuel1ORCID

Affiliation:

1. ICMCB, UMR5026, CNRS, University of Bordeaux, 33600 Pessac, France

2. School of Chemical and Biomolecular Engineering, Georgia Institute of Technology, 311 Ferst Dr NW, Atlanta, GA 30332, USA

3. BRGM, 3 Avenue Claude-Guillemin, BP 36009, CEDEX 2, 45060 Orléans, France

4. European Synchrotron Radiation Facility (ESRF), 38043 Grenoble, France

5. Institut Laue Langevin, 71 av des Martyrs, 38042 Grenoble, France

Abstract

In this study, X-ray laminography is used to monitor the evolution of a model 3D packed bed porous medium on a chip (micromodels) undergoing reactive flows. The obtained 3D images are used to compute the fluid flow patterns and develop insights into dissolution mechanisms. This study is a first proof of concept study, with controlled micromodels, and could later be extended towards deeper understanding of the dissolution and precipitation processes occurring in porous media at the microscale, mechanisms which are relevant to many industrial areas including catalysis, geochemistry, energy, and waste storage in deep geological formations, etc.

Funder

French National Research Agency

European Research Council

Publisher

MDPI AG

Subject

Process Chemistry and Technology,Chemical Engineering (miscellaneous),Bioengineering

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