Quantitative Detection of Thitsiol and Urushiol as Markers from the Gluta usitata Lacquer Tree Using HPLC

Author:

Lee Youngseo12ORCID,Lee Jihye1,Lee Kang-Bong3,Lee Won-Yong2ORCID,Lee Yeonhee1ORCID

Affiliation:

1. Advanced Analysis and Data Center, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea

2. Department of Chemistry, Yonsei University, Seoul 03722, Republic of Korea

3. Green City Technology Institute, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea

Abstract

Lacquer sap has been traditionally used in coatings and artwork. Suitable types of lacquer are required to preserve and restore artifacts. Recently, unsuitable cashew nut shell liquid (CNSL) has often been mixed with lacquer sap, so it is necessary to identify the characteristics of lacquer sap by the production area. However, research is still focused on urushiol and laccol. In this study, Myanmarese lacquer sap collected from Gluta usitata, which contains thitsiol as the main component, was analyzed by HPLC to quantify thitsiol using the standards 3-(10-phenyldecyl) benzene-1,2-diol (thitsiol 16) and 3-(8Z,11Z-pentadecadienyl)-benzenediol (urushiol 15:2) as markers, and calibration curves were plotted. The coefficients of determination (R2) for thitsiol 16 and urushiol 15:2 were 0.9985 and 0.9983, respectively. In addition, a blind test was conducted to confirm that accurate quantitative analysis was possible even when Myanmarese lacquer was mixed with lacquer from another production area, which contained urushiol as the main component, and CNSL, which contained cardol, a completely different catechol. Quantitative analysis of thitsiol 16 and urushiol 15:2 in Myanmarese lacquer using HPLC can be used to evaluate the quality of lacquer sap and for more sophisticated activities such as restoration by classifying differences in lacquer sap by the production area.

Funder

Korea Institute of Science and Technology

Publisher

MDPI AG

Subject

Chemistry (miscellaneous),Analytical Chemistry,Organic Chemistry,Physical and Theoretical Chemistry,Molecular Medicine,Drug Discovery,Pharmaceutical Science

Reference31 articles.

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2. Lu, R., and Miyakoshi, T. (2015). Lacquer Chemistry and Applications, Elsevier.

3. Impey, O. (2000). Japanische und Europäïsche Lackarbeiten: Rezeption, Adaption, Restaurierung/Japanese and European Lacquerware: Adoption, Adaptation, Conservation, Bayerisches Landesamt für Denkmalpflege.

4. Analytical pyrolysis applied to the characterisation and identification of Asian lacquers in cultural heritage samples—A review;Tamburini;J. Anal. Appl. Pyrolysis,2021

5. Htun, T. (2013). Lacquerware Journeys: The Untold Story of Burmese Lacquer, River Books Press Dist A C. [1st ed.].

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