Recent Advances in the Preparation Methods of Magnesium-Based Hydrogen Storage Materials

Author:

Xu Yaohui12ORCID,Zhou Yang3,Li Yuting4,Hao Yechen5,Wu Pingkeng6,Ding Zhao4ORCID

Affiliation:

1. Laboratory for Functional Materials, School of New Energy Materials and Chemistry, Leshan Normal University, Leshan 614000, China

2. Leshan West Silicon Materials Photovoltaic New Energy Industry Technology Research Institute, Leshan 614000, China

3. State Key Laboratory of New Textile Materials and Advanced Processing Technology, School of Textile Science and Engineering, Wuhan Textile University, Wuhan 430200, China

4. College of Materials Science and Engineering, National Engineering Research Center for Magnesium Alloys, National Innovation Center for Industry-Education Integration of Energy Storage Technology, Chongqing University, Chongqing 400044, China

5. Department of Computer Science, Illinois Institute of Technology, Chicago, IL 60616, USA

6. Department of Chemical Engineering, Illinois Institute of Technology, Chicago, IL 60616, USA

Abstract

Magnesium-based hydrogen storage materials have garnered significant attention due to their high hydrogen storage capacity, abundance, and low cost. However, the slow kinetics and high desorption temperature of magnesium hydride hinder its practical application. Various preparation methods have been developed to improve the hydrogen storage properties of magnesium-based materials. This review comprehensively summarizes the recent advances in the preparation methods of magnesium-based hydrogen storage materials, including mechanical ball milling, methanol-wrapped chemical vapor deposition, plasma-assisted ball milling, organic ligand-assisted synthesis, and other emerging methods. The principles, processes, key parameters, and modification strategies of each method are discussed in detail, along with representative research cases. Furthermore, the advantages and disadvantages of different preparation methods are compared and evaluated, and their influence on hydrogen storage properties is analyzed. The practical application potential of these methods is also assessed, considering factors such as hydrogen storage performance, scalability, and cost-effectiveness. Finally, the existing challenges and future research directions in this field are outlined, emphasizing the need for further development of high-performance and cost-effective magnesium-based hydrogen storage materials for clean energy applications. This review provides valuable insights and references for researchers working on the development of advanced magnesium-based hydrogen storage technologies.

Funder

Leshan West Silicon Materials Photovoltaic New Energy Industry Technology Research Institute

Fundamental Research Funds for the Central Universities

Opening Project of Crystalline Silicon Photovoltaic New Energy Research Institute

Leshan Normal University Research Program

Publisher

MDPI AG

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