Enhanced Lutetium Ion Sorption from Aqueous Solutions Using Activated Ion Exchangers

Author:

Jumadilov Talkybek12,Khimersen Khuangul13ORCID,Haponiuk Józef4ORCID,Totkhuskyzy Bakytgul15

Affiliation:

1. Bekturov Institute of Chemical Sciences, 106 Sh. Ualikhanov Str., Almaty 050010, Kazakhstan

2. School of Chemical Engineering, Kazakh-British Technical University, 59 Tole bi Str., Almaty 050000, Kazakhstan

3. Institute of Natural Sciences and Geography, Abai Kazakh National Pedagogical University, 13 Dostyk Ave., Almaty 050010, Kazakhstan

4. Department of Polymer Technology, Gdansk University of Technology, Gabriela Narutowicza 11/12, 80-233 Gdańsk, Poland

5. School of Pharmacy, Asfendiyarov Kazakh National Medical University, 94 Tole bi Str., Almaty 050012, Kazakhstan

Abstract

The growing demand for rare earth elements (REE) requires the search for economically viable materials to efficiently recover REE from various solutions. Our research aims to investigate the potential of using a combination of the ion exchangers Lewatit CNP LF (in H+ form) and AV-17-8 (in OH− form) as an interpolymer system, “Lewatit CNP LF@AV-17-8” (X:Y), with varying mass ratios of X:Y to enhance the sorption efficiency of lutetium ions from nitrate solution. During the study, we used a range of analytical methodologies, including gravimetry, ultraviolet-visible (UV-VIS) spectroscopy, and inductively coupled plasma optical emission spectroscopy (ICP-OES). Our findings demonstrate that the interpolymer system “Lewatit CNP LF@AV-17-8” (X:Y), with a mass ratio of 4:2, exhibited a significantly enhanced sorption rate of Lu3+ ions (42%) compared to the individual Lewatit CNP LF (6:0) (25%) and the individual AV-17-8 (0:6) (21%) over a 48 h period. Moreover, this interpolymer system has demonstrated notable conformity to the Freundlich adsorption model, highlighting its performance as an effective sorbent for lutetium (III) ions. Notably, our study presents a novel utilization of the interpolymer system “Lewatit CNP LF@AV-17-8” (4:2), with an adsorption capacity of 221.05 mg/g, to enhance the recovery of lutetium ions. The research findings demonstrate its potential for enhancing the recovery of REE.

Funder

Science Committee of the Ministry of Science and Higher Education of the Republic of Kazakhstan

Publisher

MDPI AG

Subject

Polymers and Plastics,General Chemistry

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