Degradation of Mechanical Properties of Flax/PLA Composites in Hygrothermal Aging Conditions

Abstract

The main advantage of green composites is their biodegradability, but this biodegradability can also be considered a drawback if the degradation appears during the service life of the component. Therefore, the study of the mechanical behavior of green composites after hygrothermal aging tests is necessary to analyze their degradation process. This study aims to comprehensively analyze the hygrothermal aging behavior and aging mechanism of flax-fiber-reinforced polylactic acid (PLA) biocomposites. The fully biodegradable composites are manufactured by compression molding. In addition, the influence of atmospheric-pressure plasma treatment on the mechanical properties of the biocomposite is studied. Specimens are exposed to water vapor and 40 °C environmental conditions in a stove for up to 42 days. Several specimens of each type are taken out at regular intervals and tested to examine the water absorption, mechanical properties, and thermal characterization. The results show that the stiffness was significantly reduced after 24 h due to matrix degradation, while the strength was reduced only after three weeks.