Affiliation:
1. College of Materials Science and Engineering, Taiyuan University of Technology, Taiyuan 030024, China
2. Shanxi Joint Laboratory of Coal Based Solid Waste Resource Utilization and Green Ecological Development, Taiyuan 030024, China
Abstract
The presence of lead in wastewater poses a significant threat to human health. To address this issue, coal gangue-based porous ceramics (CGPC) were developed to remove Pb2+ in wastewater. Coal gangue (CG) waste from Lvliang City, Shanxi province in China was used as raw material, and porosity was introduced through the addition of a pore-forming agent and an extrusion molding process. Properties of CGPC were characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), Brunauer–Emmett–Teller (BET) surface area analysis, Fourier transform infrared spectroscopy (FTIR), and thermogravimetric analysis (TGA) to explore its adsorption mechanism. The researchers examined the impact of pH, dosage of adsorbent, initial concentration, duration of adsorption, and temperature on the adsorption efficiency of CGPC. The CGPC of best performance had a porosity of 32.91% and compressive strength of 20.5 MPa prepared at 800 °C under nitrogen atmosphere with 10 wt% Na2CO3 pore-forming agent and 8 wt% CaO-MnO2 combined fluxing agent. The removal rate of Pb2+ in simulated lead-containing wastewater with a concentration of 200 mg/L reached 99.63%, and the maximum adsorption capacity was 32.15 mg/g. The adsorption process of Pb2+ by CGPC involves chemical adsorption and ion exchange. After being regenerated for seven cycles with 1 mol/L NaOH as the desorption agent, the removal rate of Pb2+ by CGPC still had 72%.
Funder
The Central Government Guides Local Science and Technology Development Special Fund Projects
Shanxi Province Science and Technology Major Projects
Subject
Management, Monitoring, Policy and Law,Renewable Energy, Sustainability and the Environment,Geography, Planning and Development,Building and Construction
Cited by
1 articles.
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