Screen-Printed Carbon Electrode Modified with Carbon Nanotubes and Copper Film as a Simple Tool for Determination of Trace Concentrations of Lead Ions

Author:

Grabarczyk Malgorzata1ORCID,Wawruch Agnieszka1

Affiliation:

1. Department of Analytical Chemistry, Institute of Chemical Sciences, Faculty of Chemistry, Maria Curie-Sklodowska University, 20-031 Lublin, Poland

Abstract

A copper film-modified, carboxyl-functionalized, and multi-walled carbon nanotube (MWCNT-COOH)-modified screen-printed carbon electrode (CuF/MWCNTs/SPCE) was used for lead determination using anodic stripping voltammetry. The main parameters were investigated and optimized during the development of the research procedure. The most optimal electrolyte concentrations were determined to be 0.4 M HCl and 6.3 × 10−5 M Cu(II). The optimal parameters for voltammetric stripping measurements are as follows: an accumulation potential of −0.7 V; an accumulation time of 120 s; and a pulse amplitude and pulse time of 120 mV and 2 ms, respectively. The effect of surface active substances and humic substances as potential interferents present in aqueous environmental samples was investigated. The validation of the procedure was carried out using certified reference materials, like waste water SPS-WW1 and environmental matrix TM-25.5. In addition, the developed procedure was applied to investigate lead recovery from natural environmental water, such as rivers and lakes.

Publisher

MDPI AG

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