Characteristics of Aerosol Extinction Hygroscopic Growth in the Typical Coastal City of Qingdao, China

Abstract

The aerosol hygroscopic growth (HG) characteristics in coastal areas are very complex, which is one of the main influences on the simulation accuracy of radiation transfer modeling for coastal environments. Previous studies have shown that aerosol HG characteristics are very different in open oceans and inland regions. However, the aerosol HG features in coastal areas are strongly affected by its type. In this work, an aerosol backward trajectory tracing model was used to classify the local aerosol type. Using long-term field campaign data in Qingdao (25 September 2019 to 25 October 2020), the HG characteristics of different types of aerosols (i.e., land source, sea source, and mixed aerosol) under different seasons and different atmospheric environments (i.e., pollution background and clean background) were studied. Quantitative models of aerosol HG factor were established for aerosols from different sources in different seasons and under different pollution background conditions. The major type of local aerosol is terrestrial aerosol, as the marine source only accounts for 10–20%. Seasonal HG characteristics (deliquescence point, DP) of mixed and land source aerosol vary significantly, from around RH = 60% to RH = 85%, while that of the marine aerosol is rather consistent (RH = 80%). When the atmospheric background is relatively clean, the DPs of aerosols from different sources are almost the same (about RH = 80%), but when the pollution is heavy, the DPs of terrestrial aerosols are almost 20% lower than those of marine sources. These models can be directly used to characterize the hygroscopic characteristics of atmospheric aerosols in Qingdao at specific seasons or pollution levels for radiative transfer modeling, remote sensing, and so forth.