Monitoring of Atmospheric Carbon Dioxide over a Desert Site Using Airborne and Ground Measurements

Abstract

Accurate monitoring of atmospheric carbon dioxide (CO2) is of great significance for studying the carbon cycle. Compared to ground observational sites, airborne observations cover a wider area, which help in effectively monitoring the distribution of CO2 sources and sinks. In this study, an airborne campaign was carried out in June and July 2021 to measure the atmospheric CO2 concentration over a desert site, Dunhuang, located in western China. The dry-air column-averaged CO2 mole fraction (XCO2) inversion results obtained from the Atmospheric Carbon Dioxide Lidar (ACDL) system were compared with the Orbiting Carbon Observatory 2 (OCO-2) retrievals, portable Fourier Transform Spectrometer (EM27/SUN) measurement results, and with the XCO2 estimates derived using the airborne Ultraportable Greenhouse Gas Analyzer (UGGA) and the Copernicus Atmosphere Monitoring Service (CAMS) model measurements. Moreover, the vertical CO2 profiles obtained from the OCO-2 and the CAMS datasets were also compared with the airborne UGGA measurements. OCO-2 and CAMS CO2 measurements showed a vertical distribution pattern similar to that of the aircraft-based measurements of atmospheric CO2. In addition, the relationship of atmospheric CO2 with the aerosol optical depth (AOD) was also determined and the results showed a strong and positive correlation between the two variables.