The Role of Electron Trajectories in XUV-Initiated High-Harmonic Generation

Author:

Krüger Michael,Azoury Doron,Bruner Barry,Dudovich Nirit

Abstract

High-harmonic generation spectroscopy is a powerful tool for ultrafast spectroscopy with intrinsic attosecond time resolution. Its major limitation—the fact that a strong infrared driving pulse is governing the entire generation process—is lifted by extreme ultraviolet (XUV)-initiated high-harmonic generation (HHG). Tunneling ionization is replaced by XUV photoionization, which decouples ionization from recollision. Here we probe the intensity dependence of XUV-initiated HHG and observe strong spectral frequency shifts of the high harmonics. We are able to tune the shift by controlling the instantaneous intensity of the infrared field. We directly access the reciprocal intensity parameter associated with the electron trajectories and identify short and long trajectories. Our findings are supported and analyzed by ab initio calculations and a semiclassical trajectory model. The ability to isolate and control long trajectories in XUV-initiated HHG increases the range of the intrinsic attosecond clock for spectroscopic applications.

Funder

H2020 European Research Council

Publisher

MDPI AG

Subject

Fluid Flow and Transfer Processes,Computer Science Applications,Process Chemistry and Technology,General Engineering,Instrumentation,General Materials Science

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