Quasi-2D Mn3Si2Te6 Nanosheet for Ultrafast Photonics

Author:

Lu Yan1,Zhou Zheng2,Kan Xuefen1,Yang Zixin3,Deng Haiqin3,Liu Bin4,Wang Tongtong4,Liu Fangqi4,Liu Xueyu1,Zhu Sicong4,Yu Qiang23,Wu Jian3ORCID

Affiliation:

1. School of Transportation Engineering, Jiangsu Shipping College, Nantong 226010, China

2. CAS Key Laboratory of Nanophotonic Materials and Devices & Key Laboratory of Nanodevices and Applications, i-Lab, Suzhou Institute of Nano-Tech and Nano-Bionics (SINANO), Chinese Academy of Sciences, Suzhou 215123, China

3. College of Advanced Interdisciplinary Studies, National University of Defense Technology, Changsha 410073, China

4. College of Science and Key Laboratory for Ferrous Metallurgy, Resources Utilization of Ministry of Education, Wuhan University of Science and Technology, Wuhan 430081, China

Abstract

The magnetic nanomaterial Mn3Si2Te6 is a promising option for spin-dependent electronic and magneto-optoelectronic devices. However, its application in nonlinear optics remains fanciful. Here, we demonstrate a pulsed Er-doped fiber laser (EDFL) based on a novel quasi-2D Mn3Si2Te6 saturable absorber (SA) with low pump power at 1.5 μm. The high-quality Mn3Si2Te6 crystals were synthesized by the self-flux method, and the ultrathin Mn3Si2Te6 nanoflakes were prepared by a simple mechanical exfoliation procedure. To the best of our knowledge, this is the first time laser pulses have been generated using quasi-2D Mn3Si2Te6. A stable pulsed laser at 1562 nm with a low threshold pump power of 60 mW was produced by integrating the Mn3Si2Te6 SA into an EDFL cavity. The maximum power of the output pulse is 783 μW. The repetition rate can vary from 24.16 to 44.44 kHz, with corresponding pulse durations of 5.64 to 3.41 µs. Our results indicate that the quasi-2D Mn3Si2Te6 is a promising material for application in ultrafast photonics.

Funder

China Postdoctoral Science Foundation

Hubei Province Key Laboratory of Systems Science in Metallurgical Process, Wuhan University of Science and Technology

Jiangsu Funding Program for Excellent Postdoctoral Talent

Science and Technology Program Project of Nantong City

Science and Technology Project of Jiangsu Shipping College

Publisher

MDPI AG

Subject

General Materials Science,General Chemical Engineering

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