Review on Microreactors for Photo-Electrocatalysis Artificial Photosynthesis Regeneration of Coenzymes

Author:

Liu Haixia1,Sun Rui2,Yang Yujing1,Zhang Chuanhao1,Zhao Gaozhen1,Zhang Kaihuan3ORCID,Liang Lijuan45,Huang Xiaowen1ORCID

Affiliation:

1. Department of Bioengineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250300, China

2. Jiaxing Key Laboratory of Biosemiconductors, Xiangfu Laboratory, Jiashan 314102, China

3. 2020 X-Lab, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai 200050, China

4. State Key Laboratory of Transducer Technology, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai 200050, China

5. Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China

Abstract

In recent years, with the outbreak of the global energy crisis, renewable solar energy has become a focal point of research. However, the utilization efficiency of natural photosynthesis (NPS) is only about 1%. Inspired by NPS, artificial photosynthesis (APS) was developed and utilized in applications such as the regeneration of coenzymes. APS for coenzyme regeneration can overcome the problem of high energy consumption in comparison to electrocatalytic methods. Microreactors represent a promising technology. Compared with the conventional system, it has the advantages of a large specific surface area, the fast diffusion of small molecules, and high efficiency. Introducing microreactors can lead to more efficient, economical, and environmentally friendly coenzyme regeneration in artificial photosynthesis. This review begins with a brief introduction of APS and microreactors, and then summarizes research on traditional electrocatalytic coenzyme regeneration, as well as photocatalytic and photo-electrocatalysis coenzyme regeneration by APS, all based on microreactors, and compares them with the corresponding conventional system. Finally, it looks forward to the promising prospects of this technology.

Funder

National Key Research and Development Program of China

National Natural Science Foundation of China

Shandong Provincial Key Research and Development Project

Shandong Provincial Natural Science Foundation

Talent Research Project of Qilu University of Technology

Publisher

MDPI AG

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