Investigating the Long-Term Variation Trends of Absorbing Aerosols over Asia by Using Multiple Satellites

Abstract

Absorbing aerosols, consisting of smoke (black carbon (BC) and other organics) and dust (from windblown sources), can have a strong warming effect on the climate and impact atmospheric circulation due to localized heating. To investigate the spatiotemporal and vertical changes of absorbing aerosols across Asia, collocation data from OMI, MODIS, and CALIPSO were used to compare two periods: 2006–2013 and 2014–2021. This study revealed a significant temporal and spatial contrast of aerosol loading over the study region, with a drop in total aerosol concentration and anthropogenic smoke concentration recorded across the Eastern China region (all seasons) and a concurrent increase in the Indian sub-continent region (especially in autumn). The range of aerosol diffusion is affected by the height of the smoke and aerosol plumes, as well as the wind force, and is dispersed eastwards because of the Hadley circulation patterns in the Northern Hemisphere. Smoke from Southeast Asia typically rises to a height of 3 km and affects the largest area in contrast to other popular anthropogenic zones, where it is found to be around 1.5–2 km. The dust in Inner Mongolia had the lowest plume height of 2 km (typically in spring) compared to other locations across the study region where it reached 2–5 km in the summer. This study showed, by comparison with AERONET measurements, that combining data from MODIS and OMI generates more accuracy in detecting aerosol AOD from smoke than using the instruments singularly. This study has provided a comprehensive assessment of absorbing aerosol in Asia by utilizing multiplatform remote-sensed data and has summarized long-term changes in the spatiotemporal distribution and vertical structure of absorbing aerosols.