Identification and Mapping of Three Distinct Breakup Morphologies in the Turbulent Inertial Regime of Emulsification—Effect of Weber Number and Viscosity Ratio

Abstract

Turbulent emulsification is an important unit operation in chemical engineering. Due to its high energy cost, there is substantial interest in increasing the fundamental understanding of drop breakup in these devices, e.g., for optimization. In this study, numerical breakup experiments are used to study turbulent fragmentation of viscous drops, under conditions similar to emulsification devices such as high-pressure homogenizers and rotor-stator mixers. The drop diameter was kept larger than the Kolmogorov length scale (i.e., turbulent inertial breakup). When varying the Weber number (We) and the disperse-to-continuous phase viscosity ratio in a range applicable to emulsification, three distinct breakup morphologies are identified: sheet breakup (large We and/or low viscosity ratio), thread breakup (intermediary We and viscosity ratio > 5), and bulb breakup (low We). The number and size of resulting fragments differ between these three morphologies. Moreover, results also confirm previous findings showing drops with different We differing in how they attenuate the surrounding turbulent flow. This can create ‘exclaves’ in the phase space, i.e., narrow We-intervals, where drops with lower We break and drops with higher We do not (due to the latter attenuating the surrounding turbulence stresses more).