Author:
Liu Wenxian,Qin Zhengguang,Dai Xiaojing,Meng Shibo,Niu Xinxin,Shi Wenhui,Wu Fangfang,Cao Xiehong
Abstract
Urea electrolysis is regarded as a prospective method for energy-saving hydrogen production. However, the practical application of this technology is limited by the lack of high-performance bifunctional catalysts for hydrogen evolution reaction (HER) and urea oxidation reaction (UOR). Herein, a heterostructure catalyst composed of NiFe layered double hydroxide (LDH) and sulfides (NiFe LDH-NiFeSx/NF) catalysts is prepared via a simple one-step hydrothermal approach. Remarkably, the prepared NiFe LDH-NiFeSx/NF required 138 mV and 1.34 V to achieve 10 mA cm−2 for HER and UOR in 1 M KOH and 0.33 M urea, respectively. Furthermore, when NiFe LDH-NiFeSx/NF is used as a cathode for urea electrolysis, only 1.44 V is required at 10 mA cm−2, which is much lower than the 1.53 V needed for overall water splitting.
Funder
National Natural Science Foundation of China
Zhejiang Provincial Natural Science Foundation of China
Fundamental Research Funds for the Provincial Universities of Zhejiang
Leading Innovative and Entrepreneur Team Introduction Program of Zhejiang
Subject
Energy (miscellaneous),Energy Engineering and Power Technology,Renewable Energy, Sustainability and the Environment,Electrical and Electronic Engineering,Control and Optimization,Engineering (miscellaneous),Building and Construction
Cited by
4 articles.
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