Ion-Selective Scattering Studied Using the Variable-Energy Electron Irradiation in the Ba0.2K0.8Fe2As2 Superconductor

Author:

Cho Kyuil12ORCID,Kończykowski Marcin3ORCID,Tanatar Makariy A.14ORCID,Mazin Igor I.5ORCID,Liu Yong16ORCID,Lograsso Thomas A.1ORCID,Prozorov Ruslan14ORCID

Affiliation:

1. Ames National Laboratory, Ames, IA 50011, USA

2. Department of Physics, Hope College, Holland, MI 49423, USA

3. Laboratoire des Solides Irradiés, CEA/DRF/IRAMIS, École Polytechnique, CNRS, Institut Polytechnique de Paris, F-91128 Palaiseau, France

4. Department of Physics & Astronomy, Iowa State University, Ames, IA 50011, USA

5. Department of Physics & Astronomy and Quantum Science & Engineering Center, George Mason University, Fairfax, VA 22030, USA

6. Crystal Growth Facility, Institute of Physics, École Polytechnique Fédérale de Lausanne, CH-1015 Lausanne, Switzerland

Abstract

Low-temperature variable-energy electron irradiation was used to induce non-magnetic disorder in a single crystal of a hole-doped iron-based superconductor, Ba1−xKxFe2As2, x = 0.80. To avoid systematic errors, the beam energy was adjusted non-consequently for five values between 1.0 and 2.5 MeV when sample resistance was measured in situ at 22 K. For all energies, the resistivity raises linearly with the irradiation fluence suggesting the creation of uncorrelated dilute point-like disorder (confirmed by simulations). The rate of the resistivity increase peaks at energies below 1.5 MeV. Comparison with calculated partial cross-sections points to the predominant creation of defects in the iron sublattice. Simultaneously, superconducting Tc, measured separately between the irradiation runs, is monotonically suppressed as expected, since it depends on the total scattering rate, hence on the total cross-section, which is a monotonically increasing function of the energy. Our work experimentally confirms an often-made assumption of the dominant role of the iron sub-lattice in iron-based superconductors.

Funder

U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division

Iowa State University

École Polytechnique

Publisher

MDPI AG

Subject

General Materials Science

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