Mid-Infrared Hollow-Core Fiber Based Flexible Longitudinal Photoacoustic Resonator for Photoacoustic Spectroscopy Gas Sensing

Abstract

Photoacoustic spectroscopy (PAS) has received extensive attention in optical gas sensing due to the advantages of high sensitivity, gas selectivity, and online detection. Here, a mid-infrared hollow-core fiber (HCF) based flexible longitudinal photoacoustic resonator for PAS-based gas sensing is proposed and theoretically demonstrated. A mid-infrared anti-resonant HCF is designed to innovatively replace the traditional metallic acoustic resonator and obtain a flexible photoacoustic cell in PAS. Optical transmission characteristics of the HCF are analyzed and discussed, achieving single mode operation with below 1 dB/m confinement loss between 3 and 8 μm and covering strong absorptions of some hydrocarbons and carbon oxides. With varied bending radii from 10 mm to 200 mm, the optical mode could be maintained in the hollow core. Based on the photoacoustic effect, generated acoustic mode distributions in the HCF-based flexible photoacoustic resonator are analyzed and compared. Results show that the PAS-based sensor has a stable and converged acoustic profile at the resonant frequency of around 16,787 Hz and a favorable linear response to light source power and gas concentration. The proposed novel photoacoustic resonator using HCF presents bring potential for advanced flexible PAS-based gas detection.