Rise and Fall of Anderson Localization by Lattice Vibrations: A Time-Dependent Machine Learning Approach

Author:

Zimmermann Yoel12ORCID,Keski-Rahkonen Joonas23ORCID,Graf Anton M.34ORCID,Heller Eric J.23ORCID

Affiliation:

1. Department of Chemistry and Applied Biosciences, ETH Zurich, 8093 Zurich, Switzerland

2. Department of Physics, Harvard University, Cambridge, MA 02138, USA

3. Department of Chemistry and Chemical Biology, Harvard University, Cambridge, MA 02138, USA

4. Harvard John A. Paulson School of Engineering and Applied Sciences, Harvard University, Cambridge, MA 02138, USA

Abstract

The intricate relationship between electrons and the crystal lattice is a linchpin in condensed matter, traditionally described by the Fröhlich model encompassing the lowest-order lattice-electron coupling. Recently developed quantum acoustics, emphasizing the wave nature of lattice vibrations, has enabled the exploration of previously uncharted territories of electron–lattice interaction not accessible with conventional tools such as perturbation theory. In this context, our agenda here is two-fold. First, we showcase the application of machine learning methods to categorize various interaction regimes within the subtle interplay of electrons and the dynamical lattice landscape. Second, we shed light on a nebulous region of electron dynamics identified by the machine learning approach and then attribute it to transient localization, where strong lattice vibrations result in a momentary Anderson prison for electronic wavepackets, which are later released by the evolution of the lattice. Overall, our research illuminates the spectrum of dynamics within the Fröhlich model, such as transient localization, which has been suggested as a pivotal factor contributing to the mysteries surrounding strange metals. Furthermore, this paves the way for utilizing time-dependent perspectives in machine learning techniques for designing materials with tailored electron–lattice properties.

Funder

Harvard Quantum Initiative

Oskar Huttunen Foundation

ETH Zurich

Publisher

MDPI AG

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