Effect of Co-Doping on the Magnetic Ground State of the Heavy-Fermion System CeCu2Ge2 Studied by Neutron Diffraction

Author:

Tripathi Rajesh12ORCID,Khalyavin Dmitry1ORCID,Sharma Shivani1,Adroja Devashibhai Thakarshibhai13ORCID,Hossain Zakir2

Affiliation:

1. ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot OX11 0QX, Oxon, UK

2. Department of Physics, Indian Institute of Technology, Kanpur 208016, India

3. Highly Correlated Matter Research Group, Physics Department, University of Johannesburg, P.O. Box 524, Auckland Park 2006, South Africa

Abstract

The antiferromagnetic phase transition of the heavy-fermion system Ce(Cu1−xCox)2Ge2 for x = 0.05 and 0.2, showing up in specific heat, magnetic susceptibility, and muon spin relaxation (μSR) data, has been further investigated. The neutron diffraction (ND) results show that Co-doping drastically reduces the moment size of Ce, without a qualitative change in the magnetic structure of the undoped compound CeCu2Ge2. An incommensurate magnetic propagation vector k = (0.2852, 0.2852, 0.4495) with a cycloidal magnetic structure with a Ce moment of 0.55 μB in the ab-plane has been observed for x = 0.05. Although for x = 0.2 the specific heat and magnetic susceptibility data reflect a phase transition with a broad peak and the muon relaxation rate shows a sharp peak at T = 0.9 K, our ND data dismiss the possibility of a long-range magnetic ordering down to 50 mK. The ND data, along with previously reported results for x = 0.2, are interpreted in terms of the reduced ordered state magnetic moments of the Ce3+ ion by Kondo screening and the presence of dynamical short-range magnetic correlations.

Funder

Department of Science and Technology

Jawaharlal Nehru Centre for Advanced Scientific Research

Royal Society of London and EPSRC-UK

Publisher

MDPI AG

Subject

Materials Chemistry,Chemistry (miscellaneous),Electronic, Optical and Magnetic Materials

Cited by 1 articles. 订阅此论文施引文献 订阅此论文施引文献,注册后可以免费订阅5篇论文的施引文献,订阅后可以查看论文全部施引文献

1. Magnetic and Magnetoelectric Materials;Magnetochemistry;2024-02-01

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