Lithium-Ion Battery Thermal Runaway: Experimental Analysis of Particle Deposition in Battery Module Environment

Author:

Hoelle Sebastian12ORCID,Kim Hyojeong23ORCID,Zimmermann Sascha2ORCID,Hinrichsen Olaf14ORCID

Affiliation:

1. Department of Chemistry, TUM School of Natural Sciences, Technical University of Munich, Lichtenbergstraße 4, 85748 Garching near Munich, Germany

2. BMW Group, 80937 Munich, Germany

3. Institute for Applied Materials (IAM-AWP), Karlsruhe Institute of Technology, 76344 Eggenstein-Leopoldshafen, Germany

4. Catalysis Research Center, Technical University of Munich, Ernst-Otto-Fischer-Straße 1, 85748 Garching near Munich, Germany

Abstract

In this paper, a novel experimental setup to quantify the particle deposition during a lithium-ion battery thermal runaway (TR) is proposed. The setup integrates a single prismatic battery cell into an environment representing similar conditions as found for battery modules in battery packs of electric vehicles. In total, 86 weighing plates, positioned within the flow path of the vented gas and particles, can be individually removed from the setup in order to determine the spatial mass distribution of the deposited particles. Two proof-of-concept experiments with different distances between cell vent and module cover are performed. The particle deposition on the weighing plates as well as the particle size distribution of the deposited particles are found to be dependent on the distance between cell vent and cover. In addition, the specific heat capacity of the deposited particles as well as the jelly roll remains are analyzed. Its temperature dependency is found to be comparable for both ejected particles and jelly roll remains. The results of this study help researches and engineers to gain further insights into the particle ejection process during TR. By implementing certain suggested improvements, the proposed experimental setup may be used in the future to provide necessary data for simulation model validation. Therefore, this study contributes to the improvement of battery pack design and safety.

Publisher

MDPI AG

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