Recent Advances in All-Solid-State Lithium–Oxygen Batteries: Challenges, Strategies, Future

Author:

Pakseresht Sara1ORCID,Celik Mustafa23ORCID,Guler Aslihan2,Al-Ogaili Ahmed Waleed Majeed2ORCID,Kallio Tanja1ORCID

Affiliation:

1. Department of Chemistry and Materials Science, School of Chemical Engineering, Aalto University, 02150 Espoo, Finland

2. Sakarya University Research, Development, and Application Center (SARGEM), Esentepe Campus, Sakarya 54050, Türkiye

3. Engineering Faculty, Department of Metallurgical and Materials Engineering, Esentepe Campus, Sakarya University, Sakarya 54050, Türkiye

Abstract

Digital platforms, electric vehicles, and renewable energy grids all rely on energy storage systems, with lithium-ion batteries (LIBs) as the predominant technology. However, the current energy density of LIBs is insufficient to meet the long-term objectives of these applications, and traditional LIBs with flammable liquid electrolytes pose safety concerns. All-solid-state lithium–oxygen batteries (ASSLOBs) are emerging as a promising next-generation energy storage technology with potential energy densities up to ten times higher than those of current LIBs. ASSLOBs utilize non-flammable solid-state electrolytes (SSEs) and offer superior safety and mechanical stability. However, ASSLOBs face challenges, including high solid-state interface resistances and unstable lithium-metal anodes. In recent years, significant progress has been proceeded in developing new materials and interfaces that improve the performance and stability of ASSLOBs. This review provides a comprehensive overview of the recent advances and challenges in the ASSLOB technology, including the design principles and strategies for developing high-performance ASSLOBs and advances in SSEs, cathodes, anodes, and interface engineering. Overall, this review highlights valuable insights into the current state of the art and future directions for ASSLOB technology.

Publisher

MDPI AG

Subject

Electrical and Electronic Engineering,Electrochemistry,Energy Engineering and Power Technology

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