PVB Nanocomposites as Energy Directors in Ultrasonic Welding of Epoxy Composites

Abstract

Ultrasonic welding (UW) is a well-established technique for joining thermoplastic composites and has recently been utilized in the aerospace and automotive industries. In the case of thermoset composites (TSCs), a polymer-based material placed at the welding interface called an energy director (ED) is required. The choice of the coupling layer material is linked to several requirements, such as processing temperature, high adhesion to the thermoset composites (TSCs) adherend and mechanical strength of the resulting welded joints. In this work, the authors investigated the possibility of using Poly-vinyl-butyral (PVB) reinforced with graphite nanoplatelets (GNPs) as a coupling layer in the UW of TSC adherents. The effect of GNPs aspect ratio and content on the weldability of carbon fiber-reinforced plastics (CFRP) has been investigated. PVB/GNPs nanocomposites with different filler contents (from 0.5 wt% to 2 wt%) and different aspect ratios (100 and 2100) have been fabricated. The influence of the viscoelastic properties of the flat EDs on weldability has been assessed. Finally, an improvement of lap shear strength (LSS) of 80% was found for nanocomposites with 0.5 wt% of high-aspect-ratio GNPs with respect to neat PVB. The use of high damping nanocomposites as coupling materials for TSCs paves the way for a new generation of EDs in UW.