Study on Denitration Performance of Mn-Ce/TiO2 Low-Temperature SCR Catalyst

Author:

Liu Ran1,Liu Yanting1,Gao Yanjia12,Hu Qian1

Affiliation:

1. College of Metallurgy and Energy, North China University of Technology, Tangshan 063200, China

2. Chengde Vanadium & Titanium New Material Co., Ltd., Chengde 067102, China

Abstract

Low sintering flue gas temperatures and large temperature fluctuations require the development of low-temperature and efficient SCR (selective catalytic reduction) catalysts suitable for the sintering process. It has been shown that modified Mn-Ce/TiO2 catalysts have good denitration capability and have potential commercial use. In this experiment, TiO2-loaded Mn and Ce SCR catalysts were prepared using the impregnation method, and a series of characterizations of the samples were carried out to illustrate the effect of the active material on the denitration efficiency. The kinetic analysis provides theoretical as well as data support for the subsequent optimization of the SCR catalysts. The results show that the denitration efficiency of the catalysts can reach 93.86% when the Mn content is 10% and the Ce content is 3%. The doping of active substances can increase the specific surface area, total pore volume and average aperture of the catalysts and improve the adsorption capacity of the catalysts.

Funder

National Natural Science Foundation of China

Hebei Natural Science Foundation High-end Iron and Steel Metallurgy Joint Fund

Publisher

MDPI AG

Subject

General Materials Science,Metals and Alloys

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