Challenges and Solutions for Low-Temperature Lithium–Sulfur Batteries: A Review

Author:

Liu Yiming1ORCID,Qin Tian1,Wang Pengxian1ORCID,Yuan Menglei2ORCID,Li Qiongguang34,Feng Shaojie3

Affiliation:

1. Queen Mary University of London Engineering School, Northwestern Polytechnical University, Xi’an 710129, China

2. State Key Laboratory of Solidification Processing, Center for Nano Energy Materials, School of Materials Science and Engineering, Northwestern Polytechnical University, Xi’an 710072, China

3. Anhui Province International Research Center on Advanced Building Materials, School of Materials and Chemical Engineering, Anhui Jianzhu University, Hefei 230601, China

4. Anhui Institute of Strategic Study on Carbon Dioxide Emissions Peak and Carbon Neutrality in Urban-Rural Development, Anhui Jianzhu University, Hefei 230601, China

Abstract

The lithium–sulfur (Li-S) battery is considered to be one of the attractive candidates for breaking the limit of specific energy of lithium-ion batteries and has the potential to conquer the related energy storage market due to its advantages of low-cost, high-energy density, high theoretical specific energy, and environmental friendliness issues. However, the substantial decrease in the performance of Li-S batteries at low temperatures has presented a major barrier to extensive application. To this end, we have introduced the underlying mechanism of Li-S batteries in detail, and further concentrated on the challenges and progress of Li-S batteries working at low temperatures in this review. Additionally, the strategies to improve the low-temperature performance of Li-S batteries have also been summarized from the four perspectives, such as electrolyte, cathode, anode, and diaphragm. This review will provide a critical insight into enhancing the feasibility of Li-S batteries in low-temperature environments and facilitating their commercialization.

Funder

Anhui Jianzhu University

Anhui Province International Research Center on Advanced Building Materials

Anhui Institute of Strategic Study on Carbon Dioxide Emissions Peak and Carbon Neutrality in Urban–Rural Development

Publisher

MDPI AG

Subject

General Materials Science

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