Irradiation Characteristics of Non-Impregnated Micropore Graphite for Use in Molten Salt Nuclear Reactors

Author:

Lian Pengfei12,Li Pengda23,Huang Hefei3ORCID,Song Jinliang34,Tang Zhongfeng34ORCID,Liu Zhanjun14

Affiliation:

1. Key Laboratory of Carbon Materials, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan 030001, China

2. University of Chinese Academy of Sciences, Beijing 100049, China

3. Shanghai Institute of Applied Physics, Chinese Academy of Sciences, Shanghai 201800, China

4. Dalian National Laboratory for Clean Energy, Dalian 116023, China

Abstract

Non-impregnated small-pore graphite (NSPG), which has a compact microstructure and is used in molten salt reactors (MSRs), was prepared by a novel process. The pore diameter of NSPG was reduced to ~800 nm. The irradiation evaluation of NSPG was carried out by 7 MeV Xe26+ ion irradiation. The microstructural changes of NSPG were investigated with IG-110 as a comparison. The graphitization degree of NSPG was higher than that of IG-110, though it was not subjected to an impregnation process. Under low-dose ion irradiation (<2.5 dpa), the microscopic morphology of the NSPG changes in a small magnitude, and the lamellar structure of graphite remains within the scale of more than a dozen nanometers, which exhibits a better resistance to irradiation. With the increase in irradiation dose, the accumulation of defects leads the graphite toward amorphization, which shows consistency with IG-110. This study provides an efficient and low-cost method for the preparation of graphite for MSR, and investigates the damage behavior of graphite, which is of great significance in accumulating data for the development of MSR nuclear graphite and the optimal design of graphite materials.

Funder

National Natural Science Foundation of China

Institute of Coal Chemistry, Chinese Academy of Sciences

DNL Cooperation Fund, CAS

Publisher

MDPI AG

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