Quest for Double Möbius Aromaticity

Author:

Sarmah Kangkan1,Guha Ankur K.1ORCID

Affiliation:

1. Advanced Computational Chemistry Centre, Department of Chemistry Cotton University Panbazar, Guwahati, Assam INDIA- 781001

Abstract

AbstractNeutral four‐membered rings with 4n electrons are generally Hückel antiaromatic. On the other hand, 4n electron system can also be Möbius aromatic, although identification has escaped so far. A recent study of double Möbius aromaticity has been put forwarded in the D2h symmetric singlet ground state of four member Pa2B2 ring. Although interesting, but the synthesis possesses a significant challenge as Pa is rare, highly radioactive and toxic. Herein, a synthetically viable four membered Rh2B2 cluster is proposed which contains double Möbius aromaticity. Interestingly, the three membered RhB2 cluster also possess Möbius aromaticity and is the smallest ring to show such phenomenon.

Publisher

Wiley

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