Nitrogen Fixation by Manganese Complexes – Waiting for the Rush?

Author:

Le Dé Quentin1,Valyaev Dmitry A.1ORCID,Simonneau Antoine1ORCID

Affiliation:

1. LCC–CNRS Université de Toulouse, CNRS, UPS 205 route de Narbonne BP44099, F-31077 Toulouse cedex 4 France

Abstract

AbstractManganese is currently experiencing a great deal of attention in homogeneous catalysis as a sustainable alternative to platinum group metals due to its abundance, affordable price and low toxicity. While homogeneous nitrogen fixation employing well‐defined transition metal complexes has been an important part of coordination chemistry, manganese derivatives have been only sporadically used in this research area. In this contribution, the authors systematically cover manganese organometallic chemistry related to N2 activation spanning almost 60 years, identify apparent pitfalls and outline encouraging perspectives for its future development.

Funder

H2020 European Research Council

Publisher

Wiley

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