Research on etalon‐free CO2 measurement based on direct absorption signal fitting

Author:

Yang Yan1,Guo Songjie1,Li Jiatong1,Wei Youxing1,Lu Zhimin12,Xing Xiwen3,Ren Wei4,Zhang Xiang5,Yao Shunchun12ORCID

Affiliation:

1. School of Electric Power South China University of Technology Guangzhou China

2. Guangdong Province Key Laboratory of Efficient and Clean Energy Utilization Guangzhou China

3. College of Life Science and Technology Jinan University Guangzhou China

4. Department of Mechanical and Automation Engineering Chinese University of Hong Kong Hong Kong China

5. South China National Centre of Metrology Guangzhou China

Abstract

AbstractThe emission of carbon dioxide (CO2) by thermal power plants is the main factor leading to the greenhouse effect. The measurement of CO2 is of great significance to carbon emission data statistics. In this paper, a measurement system based on tunable diode laser absorption spectroscopy (TDLAS) was built to measure the spectrum of CO2 near 1579 nm. To simplify the experimental system, a direct absorption signal fitting method is proposed to replace etalons for time‐frequency conversion. The method was applied to the measurement of four different concentrations of CO2 in the range of 7%–16%, and the measurement results were compared with the multipeak method, another etalon‐free method. The results show that the mean relative error of the measurement results is 4.23%, which is 1.76% lower than the measurement results of the multipeak method. The experimental research provides a feasible idea to simplify the CO2 measurement system based on TDLAS.

Funder

National Natural Science Foundation of China

Innovation and Technology Commission

Publisher

Wiley

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