Graphene Oxide‐Arginine Composites: Efficient Dual Function Materials for Integrated CO<sub>2</sub> Capture and Conversion-Reference-Cited by-同舟云学术

Graphene Oxide‐Arginine Composites: Efficient Dual Function Materials for Integrated CO₂ Capture and Conversion

Published:2024-01-29 Issue:5 Volume:17 Page:
ISSN:1864-5631
Container-title:ChemSusChem
language:en
Short-container-title:ChemSusChem

Author:

Mantovani Sebastiano¹²,Pintus Angela²,Kovtun Alessandro²,Gondolini Angela³,Casadio Simone³⁴,Sanson Alessandra³,Marforio Tainah D.¹⁵,Calvaresi Matteo¹⁵,Rancan Marzio⁶,Armelao Lidia⁴⁷,Bertuzzi Giulio¹⁵,Melucci Manuela²,Bandini Marco¹⁵^ORCID

Affiliation:

1. Dipartimento di Chimica “Giacomo Ciamician” Alma Mater Studiorum – Università di Bologna via P. Gobetti 85 40129 Bologna Italy

2. The Institute for Organic Synthesis and Photoreactivity (ISOF) National Research Council (CNR) via P. Gobetti 101 40129 Bologna Italy

3. Institute of Science, Technology and Sustainability for Ceramics (ISSMC, former ISTEC) National Research Council (CNR) via Granarolo, 64 48018 Faenza RA Italy

4. Department of Chemical Sciences University of Padova via Marzolo 1 35131 Padova Italy

5. Center for Chemical Catalysis – C3 Alma Mater Studiorum – Università di Bologna via R. Gobetti 85 40129 Bologna Italy

6. Institute of Condensed Matter Chemistry and Technologies for Energy (ICMATE) National Research Council (CNR) c/o Department of Chemical Sciences University of Padova via Marzolo 1 35131 Padova Italy

7. Department of Chemical Sciences and Materials Technologies (DSCTM) National Research Council (CNR) Piazzale Moro 7 00185 Roma Italy

Abstract

AbstractThe “on‐demand” capture and utilization of CO2 is effectively realized with a readily accessible dual function organic composite. The covalent and controlled derivatization of graphene oxide (GO) surface with naturally occurring arginine led to a “smart” material capable of capturing (chemisorption) CO2 from high‐purity flue‐gas as well as low‐concentration streams (i. e. direct air capture) and concomitant chemical activation toward the incorporation into cyclic carbonates. The overall integrated CO2 capture and conversion (ICCC) strategy has been fully elucidated mechanistically via dedicated computational, spectroscopic and thermal analyses.

Funder

Università di Bologna

Publisher

Wiley

Reference83 articles.

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