Graphene Oxide‐Arginine Composites: Efficient Dual Function Materials for Integrated CO2 Capture and Conversion

Author:

Mantovani Sebastiano12,Pintus Angela2,Kovtun Alessandro2,Gondolini Angela3,Casadio Simone34,Sanson Alessandra3,Marforio Tainah D.15,Calvaresi Matteo15,Rancan Marzio6,Armelao Lidia47,Bertuzzi Giulio15,Melucci Manuela2,Bandini Marco15ORCID

Affiliation:

1. Dipartimento di Chimica “Giacomo Ciamician” Alma Mater Studiorum – Università di Bologna via P. Gobetti 85 40129 Bologna Italy

2. The Institute for Organic Synthesis and Photoreactivity (ISOF) National Research Council (CNR) via P. Gobetti 101 40129 Bologna Italy

3. Institute of Science, Technology and Sustainability for Ceramics (ISSMC, former ISTEC) National Research Council (CNR) via Granarolo, 64 48018 Faenza RA Italy

4. Department of Chemical Sciences University of Padova via Marzolo 1 35131 Padova Italy

5. Center for Chemical Catalysis – C3 Alma Mater Studiorum – Università di Bologna via R. Gobetti 85 40129 Bologna Italy

6. Institute of Condensed Matter Chemistry and Technologies for Energy (ICMATE) National Research Council (CNR) c/o Department of Chemical Sciences University of Padova via Marzolo 1 35131 Padova Italy

7. Department of Chemical Sciences and Materials Technologies (DSCTM) National Research Council (CNR) Piazzale Moro 7 00185 Roma Italy

Abstract

AbstractThe “on‐demand” capture and utilization of CO2 is effectively realized with a readily accessible dual function organic composite. The covalent and controlled derivatization of graphene oxide (GO) surface with naturally occurring arginine led to a “smart” material capable of capturing (chemisorption) CO2 from high‐purity flue‐gas as well as low‐concentration streams (i. e. direct air capture) and concomitant chemical activation toward the incorporation into cyclic carbonates. The overall integrated CO2 capture and conversion (ICCC) strategy has been fully elucidated mechanistically via dedicated computational, spectroscopic and thermal analyses.

Funder

Università di Bologna

Publisher

Wiley

Reference83 articles.

1.  

2. H. Ritchie M. Roser “CO₂ and Greenhouse Gas Emissions”. Published online at OurWorldInData.org. Retrieved from:https://ourworldindata.org/co2-and-other-greenhouse-gas-emissions 2017;

3. Atmospheric CO 2 : Principal Control Knob Governing Earth’s Temperature

4. The role of CO2 capture and utilization in mitigating climate change

5. New directions of technologies pointing the way to a sustainable global society

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