Smart anti‐fouling and self‐repairing polymer brushes for efficient oil–water separation

Author:

Liu Jinhui1,Yuan Yuka1,Peng Shuoli1,Guo Liyun1,Liu Yudong1,Li Shulan1,Liu Kai2,Hua Jing1ORCID

Affiliation:

1. Key Laboratory of Rubber‐Plastics, Ministry of Education/Shandong Provincial Key Laboratory of Rubber and Plastics Qingdao University of Science and Technology Qingdao Shandong People's Republic of China

2. Beijing National Laboratory for Molecular Sciences Key Laboratory of Organic Solids Institute of Chemistry Chinese Academy of Sciences Beijing People's Republic of China

Abstract

AbstractThe increasing water pollution problem poses a demand for oil–water separation materials, but preparing separation materials with high efficiency and excellent durability remains a great challenge. In this work, we use a diblock polymer brush of polydimethylsiloxane (PDMS) and poly(N,N‐dimethylaminoethyl methacrylate) (PDMAEMA) based on cotton fabric to prepare oil–water separation membranes with high efficiency, good durability, and intelligent self‐repairing properties. Lubricating PDMS brushes reduces the fouling adhesion due to its low surface energy and high flexibility. pH‐responsive PDMAEMA brushes provide good hydrophobicity and an intelligent self‐repairing effect. The prepared Co‐PDMS‐PDMAEMA has high oil flux (>30,000 L m−2 h−1) and high separation efficiency (>99%) even after 10 cycles and its surface character can be recovered under acidic conditions. Overall, the modified cotton fabric made by such a versatile technique is promising in oil–water separation.

Funder

National Natural Science Foundation of China

Publisher

Wiley

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