Unveiling All‐Optical Switching Phenomenon in Anthracene Derivatives: A Comprehensive Study on Optical and Nonlinear Optical Multifunctionality

Author:

Szukalski Adam1ORCID,Zajac Dorota1,Pardus Natasza1,Karout Houda El23,Krawczyk Przemyslaw4,Sahraoui Bouchta3

Affiliation:

1. Institute of Advanced Materials Wroclaw University of Science and Technology Wybrzeze Wyspianskiego 27 Wroclaw 50–370 Poland

2. Univ Angers, CNRS MOLTECH‐ANJOU, SFR MATRIX Angers F‐49000 France

3. Univ Angers, LPHIA SFR MATRIX Angers F‐49000 France

4. Faculty of Pharmacy Nicolaus Copernicus University Collegium Medicum Kurpińskiego 5 Bydgoszcz 85–950 Poland

Abstract

AbstractIn this study, it is considered three anthracene derivatives, characterized meticulously in terms of their chemical structure and product purity. Extensive quantum chemical calculations are conducted to elucidate their optical and nonlinear optical properties, shedding light on the mechanism of photoinduced conformational transformation, a pivotal discovery in this research. Experimental analyses encompassed fundamental optical properties and advanced nonlinear optical phenomena, including z‐scan experiments, second harmonic generation (SHG), and third harmonic generation (THG). Remarkably, a groundbreaking all‐optical switching phenomenon in these materials is experimentally validated, marking a significant advancement and contributing to their potential applications.

Funder

Wroclawskie Centrum Sieciowo-Superkomputerowe, Politechnika Wroclawska

Publisher

Wiley

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