Affiliation:
1. School of Materials Science and Engineering Changchun University of Science and Technology Changchun 130022 China
2. Engineering Research Center of Optoelectronic Functional Materials Ministry of Education Changchun 130022 China
Abstract
AbstractThe low gain in the presence of a single transverse external electric field limits the application of metal‐semiconductor‐metal (MSM) photodetectors. Here, a longitudinal built‐in electric field by spin‐coating CH3NH3PbI3:PC61BM on the electrode region of an Au/ZnO MSM photodetector, which constitutes a vertically crossed composite electric field with a transverse external electric field, is constructed. In this case, the transverse electric field collects the electrons, and the longitudinal electric field separates them. Based on this novel electric field structure, carrier multiplication at lower voltage conditions is achieved. Compared to the low voltage, there is a significant amplification effect when the voltage reaches 7 V. The responsivity is increased ≈270 times for UV–vis wavelengths, escalating from ≈0.02 to ≈5.4 A W−1. This study provides a novel carrier transport control scheme for high‐gain perovskite‐based photodetectors.
Funder
Jilin Provincial Scientific and Technological Development Program
National Natural Science Foundation of China