Application of Energy‐Resolving Neutron Imaging to Major‐Component Analyses of Materials Using Four‐Channel Superconducting Detector

Author:

Vu The Dang1ORCID,Shishido Hiroaki2ORCID,Aizawa Kazuya3,Oku Takayuki3ORCID,Oikawa Kenichi3ORCID,Harada Masahide3,Kojima Kenji M.4ORCID,Miyajima Shigeyuki5ORCID,Soyama Kazuhiko3,Koyama Tomio1,Hidaka Mutsuo6,Suzuki Soh Y.7ORCID,Tanaka Manobu M.8,Machida Masahiko9,Kawamata Shuichi1,Ishida Takekazu1ORCID

Affiliation:

1. Division of Quantum and Radiation Engineering Osaka Metropolitan University Sakai Osaka 599‐8570 Japan

2. Department of Physics and Electronics Graduate School of Engineering, Osaka Metropolitan University Sakai Osaka 599‐8531 Japan

3. Materials and Life Science Division J‐PARC Center, Japan Atomic Energy Agency Tokai Ibaraki 319‐1195 Japan

4. Centre for Molecular and Materials Science, TRIUMF, 4004 Wesbrook Mall Vancouver British Columbia V6T 2A3 Canada

5. Advanced ICT Research Institute National Institute of Information and Communications Technology, 588‐2 Iwaoka, Nishi‐ku Kobe Hyogo 651‐2492 Japan

6. Advanced Industrial Science and Technology Tsukuba Ibaraki 305‐8568 Japan

7. Computing Research Center, Applied Research Laboratory High Energy Accelerator Research Organization (KEK) Tsukuba Ibaraki 305‐0801 Japan

8. Institute of Particle and Nuclear Studies High Energy Accelerator Research Organization (KEK) Tsukuba Ibaraki 305‐0801 Japan

9. Center for Computational Science & e‐Systems Japan Atomic Energy Agency, 178‐4‐4 Wakashiba Kashiwa Chiba 277‐0871 Japan

Abstract

We proposed a current‐biased kinetic inductance detector (CB‐KID) as a novel superconducting detector to construct a neutron transmission imager. The characteristics of a superconducting neutron detector have been systematically studied to improve a spatial resolution down to 10 in transmission imaging. In this study, we report the application of the energy‐resolving neutron imaging to investigate major components of materials by analyzing neutron transmission spectra from 1 meV to 500 keV. We succeeded in identifying that copper (Cu) and iron (Fe) are major components respectively in commercial nuts and screws as test samples with the aid of Rietveld imaging of transmission spectra (RITS) program in analyzing transmission spectra in longer wavelengths. The Ti screw was also confirmed by comparing the nuclear resonance absorption measurements and simulations in high‐energy regions. We demonstrated that our superconducting neutron detector is applicable to reveal the transmission spectra in the wide range from cold‐neutron energies to higher neutron energies even up to 500 keV. By selecting distinctive energy regions of pulsed neutrons, we succeeded in mapping the distribution of SmSn3 compound using the strong neutron absorption in samarium (Sm) and the selective nuclear‐resonance dips in Sm. By taking advantage of using CB‐KID in conducting neutron imaging, the CB‐KID method is extensively useful for various purposes in material sciences through energy‐selective neutron spectroscopy from 1 meV to 500 keV. © 2024 Institute of Electrical Engineers of Japan and Wiley Periodicals LLC.

Funder

Materials and Life Science Experimental Facility

Publisher

Wiley

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