A flexible ammonia sensor based on MXene membrane with high sensitivity

Author:

Zhao Qian12,Li Yilin2,Zhang Zhouxiaolong2,Dai Li3,Liu Xuhan4,Sun Yanhui5,Zhao Dan6,Zhu Nan12ORCID

Affiliation:

1. Cancer Hospital of Dalian University of Technology Dalian University of Technology 110042 Liaoning Province China

2. School of Chemistry Dalian University of Technology Dalian, Liaoning 116024 China

3. Second Affiliated Hospital Dalian Medical University 116023 Dalian China

4. Department of Endocrinology Dalian Municipal Central Hospital Dalian 116089 China

5. College of Information & Communication Engineering Dalian Minzu University Dalian 116600 China

6. Laboratory of Organic Electronics Department of Science and Technology Linköping University 60174 Norrköping Sweden

Abstract

AbstractAmmonia (NH3) of high concentration will pose a threat to ecological environment or human health, and exhaled NH3 is significant in disease monitoring and diagnosis. Thus, developing a highly sensitive gas sensor is significant to monitor NH3 concentration in complex environments. However, traditional NH3 sensors either need high working temperature, or face the challenge of poor conductivity/ sensitivity. In this work, NH3 sensors based on self‐assembled MXene membrane have been fabricated. As‐prepared sensors show a high sensitivity of 2.10 ppm−1 towards extremely low concentrations of NH3 (ppb level) at room temperature, attributed to large surface area and high conductivity. In addition, the sensors also display low detection limit (50 ppb), fast response time (41 s), good recoverability, long‐term stability (15 days) and excellent flexibility (1000 bending cycles) towards NH3. The results provide insights into the development of highly sensitive NH3 sensors for industrial or biomedical applications.

Funder

National Natural Science Foundation of China

Publisher

Wiley

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