Emerging Data Processing Methods for Single‐Entity Electrochemistry

Author:

Li Xinyi1,Fu Ying‐Huan1,Wei Nannan2,Yu Ru‐Jia13,Bhatti Huma1,Zhang Limin2,Yan Feng2,Xia Fan4,Ewing Andrew G.5ORCID,Long Yi‐Tao1,Ying Yi‐Lun13ORCID

Affiliation:

1. State Key Laboratory of Analytical Chemistry for Life Science, School of Chemistry and Chemical Engineering Nanjing University 210023 Nanjing P. R. China

2. School of Electronic Science and Engineering Nanjing University 210023 Nanjing P. R. China

3. Chemistry and Biomedicine Innovation Center Nanjing University 210023 Nanjing P. R. China

4. State Key Laboratory of Biogeology and Environmental Geology, Engineering Research Center of Nano-Geomaterials of Ministry of Education, Faculty of Materials Science and Chemistry China University of Geosciences 430034 Wuhan P. R. China

5. Department of Chemistry and Molecular Biology University of Gothenburg 41296 Gothenburg Sweden

Abstract

AbstractSingle‐entity electrochemistry is a powerful tool that enables the study of electrochemical processes at interfaces and provides insights into the intrinsic chemical and structural heterogeneities of individual entities. Signal processing is a critical aspect of single‐entity electrochemical measurements and can be used for data recognition, classification, and interpretation. In this review, we summarize the recent five‐year advances in signal processing techniques for single‐entity electrochemistry and highlight their importance in obtaining high‐quality data and extracting effective features from electrochemical signals, which are generally applicable in single‐entity electrochemistry. Moreover, we shed light on electrochemical noise analysis to obtain single‐molecule frequency fingerprint spectra that can provide rich information about the ion networks at the interface. By incorporating advanced data analysis tools and artificial intelligence algorithms, single‐entity electrochemical measurements would revolutionize the field of single‐entity analysis, leading to new fundamental discoveries.

Funder

National Natural Science Foundation of China

Vetenskapsrådet

H2020 European Research Council

Publisher

Wiley

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