Few‐Layer Fullerene Network for Photocatalytic Pure Water Splitting into H2 and H2O2

Author:

Wang Taotao12,Zhang Li1,Wu Jinbao1,Chen Muqing2,Yang Shangfeng1,Lu Yalin1,Du Pingwu1ORCID

Affiliation:

1. Key Laboratory of Precision and Intelligent Chemistry Anhui Laboratory of Advanced Photon Science and Technology Department of Materials Science and Engineering University of Science and Technology of China 96 Jinzhai Road Hefei Anhui Province 230026 P. R. China

2. School of Materials Science and Engineering Dongguan University of Technology Dongguan Guangdong Province 523808 P. R. China

Abstract

AbstractA few‐layer fullerene network possesses several advantageous characteristics, including a large surface area, abundant active sites, high charge mobility, and an appropriate band gap and band edge for solar water splitting. Herein, we report for the first time that the few‐layer fullerene network shows interesting photocatalytic performance in pure water splitting into H2 and H2O2 in the absence of any sacrificial reagents. Under optimal conditions, the H2 and H2O2 evolution rates can reach 91 and 116 μmol g−1 h−1, respectively, with good stability. This work demonstrates the novel application of the few‐layer fullerene network in the field of energy conversion.

Funder

National Natural Science Foundation of China

Publisher

Wiley

Subject

General Medicine

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