A Deeper Understanding of Metal Nucleation and Growth in Rechargeable Metal Batteries Through Theory and Experiment

Author:

Cooper Emily R.1ORCID,Li Ming2ORCID,Gentle Ian3ORCID,Xia Qingbing4ORCID,Knibbe Ruth1ORCID

Affiliation:

1. School of Mining and Mechanical Engineering The University of Queensland <postCode4067 Brisbane Australia

2. Central Analytical Research Facility Queensland University of Technology 4000 Brisbane Australia

3. School of Chemistry and Molecular Biosciences The University of Queensland 4067 Brisbane Australia

4. School of Chemical Engineering The University of Queensland 4067 Brisbane Australia

Abstract

AbstractLithium and sodium metal batteries continue to occupy the forefront of battery research. Their exceptionally high energy density and nominal voltages are highly attractive for cutting‐edge energy storage applications. Anode‐free metal batteries are also coming into the research spotlight offering improved safety and even higher energy densities than conventional metal batteries. However, uneven metal nucleation and growth which leads to dendrites continues to limit the commercialisation of conventional and anode‐free metal batteries alike. This review connects models and theories from well‐established fields in metallurgy and electrodeposition to both conventional and anode‐free metal batteries. These highly applicable models and theories explain the driving forces of uneven metal growth and can inform future experiment design. Finally, the models and theories that are most relevant to each anode‐related cell component are identified. Keeping these specific models and theories in mind will assist with rational design for these components.

Funder

Australian Research Council

Publisher

Wiley

Subject

General Medicine

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