Selective Oxidation of Methanol to Green Oxygenates – Feasibility Study of Fixed‐Bed and Membrane Reactors

Author:

Walter Jan P.1,Hamel Christof1

Affiliation:

1. Otto von Guericke University Magdeburg Institute of Process Engineering Universitätsplatz 2 39106 Magdeburg Germany

Abstract

AbstractA feasibility study of a conventional fixed‐bed reactor and a packed‐bed membrane reactor (PBMR) in distributor configuration is carried out for the selective oxidation of methanol to the oxygenates dimethoxymethane and methyl formate on a VOx/TiO2 catalyst. Kinetic experiments provided the reaction network and a reliable kinetic model of six main reactions involved. The PBMR offers significant advantages and potential for the formation of both target products due to an effective kinetic coupling of the oxidative dehydrogenation of methanol and the consecutive reaction steps to dimethoxymethane and methyl formate in a broad range of operation conditions.

Publisher

Wiley

Subject

Industrial and Manufacturing Engineering,General Chemical Engineering,General Chemistry

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