Application of a Scaled‐up Dielectric Barrier Discharge Reactor in the Trace Oxygen Removal in Hydrogen‐Rich Gas Mixtures at Ambient and Elevated Pressure

Author:

Wirth Philipp1ORCID,Oberste‐Beulmann Christian2,Nitsche Tim3ORCID,Muhler Martin2ORCID,Awakowicz Peter1ORCID

Affiliation:

1. Chair of Applied Electrodynamics and Plasma Technology Ruhr University Bochum Universitaetsstr. 150 44780 Bochum Germany

2. Laboratory of Industrial Chemistry Ruhr University Bochum Universitaetsstr. 150 44780 Bochum Germany

3. Fraunhofer Institute for Environmental Security and Energy Technology UMSICHT Osterfelder Str. 3 46047 Oberhausen Germany

Abstract

AbstractDielectric barrier discharges (DBDs) are frequently utilized in various gas conversion processes. For industrial applications a low flow resistance and scalability are crucial. In this study a tenfold scaled‐up reactor based on a surface dielectric barrier discharge (SDBD) was employed for the removal of oxygen traces from H2/N2/O2 gas mixtures. The conversion efficiency of the reactor with ten electrode configurations was investigated for different admixtures of O2, and high degrees of conversion were observed that decreased with increasing flow rate, but remained constant when raising the pressure to 2 bar(g). A new generator based on silicon carbide field‐effect transistors (SiC‐FETs) was used and compared to a generator based on classical metal oxide semiconductor field‐effect transistors (MOS‐FETs).

Funder

Bundesministerium für Bildung und Forschung

Publisher

Wiley

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