Splitting behavior and breakup mechanism of bubbles in the split‐and‐recombine microchannel

Abstract

AbstractSplit‐and‐recombine (SAR) microreactor is an advanced reactor for chemical process intensification. Bubble flow in the SAR microchannel is an important phenomenon that affects reaction efficiency, however drew little attention before. This study aims to explore the underlying mechanisms of bubble splitting, retraction, and breakup behaviors in a compact SAR microchannel. Two breakup flow patterns, unilateral flow and unilateral alternate flow were identified with symmetric or asymmetric splitting, respectively. Mechanism analysis indicates that the splitting symmetry issue is related to liquid slug size, viscous effect and novel retraction behavior of a splitting filament. The retraction is induced by the interconnection and unequal pressures between the splitting filaments. The correlation between normalized breakup time and Ca number confirms the Capillary‐pressure breakup mechanism for the splitting gas filaments. Two empirical correlations for the two breakup flow patterns were proposed, which illustrate the significant contribution of bubble retraction to the breakup degree.