Advances in electrolyzer design and development for electrochemical CO2 reduction

Author:

He Ruinan1,Xu Nengneng12,Hasan Israr Masood ul1,Peng Luwei13,Li Lulu1,Huang Haitao3ORCID,Qiao Jinli12ORCID

Affiliation:

1. State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Environmental Science and Engineering, Donghua University Shanghai China

2. Shanghai Institute of Pollution Control and Ecological Security Shanghai China

3. Department of Applied Physics and Research Institute for Smart Energy Hong Kong Polytechnic University Kowloon Hong Kong China

Abstract

AbstractIn view of global energy transition and environmental issues, electrochemical conversion of carbon dioxide (CO2) to high value‐added chemicals by using clean renewable electricity, as an advanced carbon capture, utilization and storage (CCUS) technology, demonstrates a promising approach to reach the carbon neutrality with additional economic benefits as well. Over the past decade, various new valid catalysts in electrochemical CO2 reduction (ECO2R) have been designed and intensively investigated. Unfortunately, constructing appropriate ECO2R electrolyzer with high conversion rate and long‐term stability to unleash the full potential benefits of electrocatalysts remains a recognized challenge, especially as it has not yet attracted attention. This review summarizes the progress of ECO2R reactor and their corresponding structure characteristics/ electrochemical performance. Besides, the current challenges and bottlenecks of CO2RR reactor are discussed. We aim to introduce the advances in ECO2R electrolyzer in detail to offer enlightenment for large‐scale industrial application of ECO2R.image

Funder

National Key Research and Development Program of China

National Natural Science Foundation of China

Fundamental Research Funds for the Central Universities

Publisher

Wiley

Subject

Materials Science (miscellaneous),Physical and Theoretical Chemistry,Chemistry (miscellaneous)

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