Carbon−Sulfur Coupling Reactions Catalyzed by Nickel(II) N‐Heterocyclic Carbene Complexes

Author:

Neshat Abdollah1ORCID,Khezri Rahimeh2,Yousefshahi Mohammad Reza1,Gholinejad Mohammad1,Varmaghani Fahimeh1

Affiliation:

1. Department of Chemistry Institute for Advanced Studies in Basic Sciences (IASBS) 444 Prof. Sobouti Blvd., Gava Zang Zanjan 45137-66731 Iran

2. Department of Chemistry Faculty of Science Persian Gulf University 75169 Bushehr Iran

Abstract

AbstractThe synthesis and characterization of Nickel(II) complexes with novel pincer‐type N‐heterocyclic carbene complexes were investigated. Nickel(II)‐NHC complexes, 7 and 8, were characterized using HR ESI‐MS, IR, UV‐Visible, and elemental analysis. The complex 7 with less sterically demanding pincer ligand was investigated in the catalytic one pot synthesis of thioethers via coupling reactions of a series of aryl and alkyl halides in the presence of thiourea. In a mixture of water and ethanol, 5 mol% of 7 catalyzed the C−S bond coupling reaction in high yields.

Publisher

Wiley

Subject

Inorganic Chemistry

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