“On‐The‐Fly” Synthesis of Self‐Supported LDH Hollow Structures Through Controlled Microfluidic Reaction‐Diffusion Conditions

Author:

Mattera Michele1,Sorrenti Alessandro2,De Gregorio Perpiñá Lidia1,Oestreicher Víctor3,Sevim Semih4,Arteaga Oriol5,Chen Xiang‐Zhong6,Pané Salvador4,Abellán Gonzalo3,Puigmartí‐Luis Josep17ORCID

Affiliation:

1. Departament de Ciència dels Materials i Química Física Institut de Química Teòrica i Computacional University of Barcelona (UB) Barcelona 08028 Spain

2. Departament de Química Inorgànica i Orgànica (Secció de Química Orgànica) University of Barcelona (UB) Barcelona 08028 Spain

3. Institute of Molecular Science University of Valencia (UVEG) c/Catedrático José Beltrán 2 Paterna 46980 Spain

4. Institute of Robotics and Intelligent Systems ETH Zurich Tannenstrasse 3 Zurich CH 8092 Switzerland

5. Departament de Fisica Aplicada PLAT group Universitat de Barcelona IN2UB Barcelona 08028 Spain

6. Institute of Optoelectronics State Key Laboratory of Photovoltaic Science and Technology Shanghai Frontiers Science Research Base of Intelligent Optoelectronics and Perception Fudan University Shanghai 200438 P. R. China

7. Institució Catalana de Recerca i Estudis Avançats (ICREA) Pg. Lluís Companys 23 Barcelona 08010 Spain

Abstract

AbstractLayered double hydroxides (LDHs) are a class of functional materials that exhibit exceptional properties for diverse applications in areas such as heterogeneous catalysis, energy storage and conversion, and bio‐medical applications, among others. Efforts have been devoted to produce millimeter‐scale LDH structures for direct integration into functional devices. However, the controlled synthesis of self‐supported continuous LDH materials with hierarchical structuring up to the millimeter scale through a straightforward one‐pot reaction method remains unaddressed. Herein, it is shown that millimeter‐scale self‐supported LDH structures can be produced by means of a continuous flow microfluidic device in a rapid and reproducible one‐pot process. Additionally, the microfluidic approach not only allows for an “on‐the‐fly” formation of unprecedented LDH composite structures, but also for the seamless integration of millimeter‐scale LDH structures into functional devices. This method holds the potential to unlock the integrability of these materials, maintaining their performance and functionality, while diverging from conventional techniques like pelletization and densification that often compromise these aspects. This strategy will enable exciting advancements in LDH performance and functionality.

Funder

Agencia Estatal de Investigación

European Research Council

Generalitat Valenciana

Publisher

Wiley

Subject

Biomaterials,Biotechnology,General Materials Science,General Chemistry

同舟云学术

1.学者识别学者识别

2.学术分析学术分析

3.人才评估人才评估

"同舟云学术"是以全球学者为主线,采集、加工和组织学术论文而形成的新型学术文献查询和分析系统,可以对全球学者进行文献检索和人才价值评估。用户可以通过关注某些学科领域的顶尖人物而持续追踪该领域的学科进展和研究前沿。经过近期的数据扩容,当前同舟云学术共收录了国内外主流学术期刊6万余种,收集的期刊论文及会议论文总量共计约1.5亿篇,并以每天添加12000余篇中外论文的速度递增。我们也可以为用户提供个性化、定制化的学者数据。欢迎来电咨询!咨询电话:010-8811{复制后删除}0370

www.globalauthorid.com

TOP

Copyright © 2019-2024 北京同舟云网络信息技术有限公司
京公网安备11010802033243号  京ICP备18003416号-3