The Coexistence of Superconductivity and Topological Order in Van der Waals InNbS2

Abstract

AbstractThe research on systems with coexistence of superconductivity and nontrivial band topology has attracted widespread attention. However, the limited availability of material platforms severely hinders the research progress. Here, it reports the first experimental synthesis and measurement of high‐quality single crystal van der Waals transition‐metal dichalcogenide InNbS2, revealing it as a topological nodal line semimetal with coexisting superconductivity. The temperature‐dependent measurements of magnetization susceptibility and electrical transport show that InNbS2 is a type‐II superconductor with a transition temperature Tc of 6 K. First‐principles calculations predict multiple topological nodal ring states close to the Fermi level in the presence of spin–orbit coupling. Similar features are also observed in the as‐synthesized BiNbS2 and PbNbS2 samples. This work provides new material platforms ANbS2 (A = In, Bi, and Pb) and uncovers their intriguing potential for exploring the interplay between superconductivity and band topology.