2D Layered Materials for Fast‐Charging Lithium‐Ion Battery Anodes

Author:

Yang Yaxiong1,Dong Ruige2,Cheng Hao34,Wang Linlin4,Tu Jibing4,Zhang Shichao3,Zhao Sihan2,Zhang Bing34,Pan Hongge15,Lu Yingying134ORCID

Affiliation:

1. Institute of Science and Technology for New Energy Xi'an Technological University Xi'an 710021 China

2. Interdisciplinary Center for Quantum Information State Key Laboratory of Silicon Materials and Zhejiang Province Key Laboratory of Quantum Technology and Device Department of Physics Zhejiang University Hangzhou 310058 China

3. State Key Laboratory of Chemical Engineering, Institute of Pharmaceutical Engineering, College of Chemical and Biological Engineering Zhejiang University Hangzhou 310027 China

4. ZJU‐Hangzhou Global Scientific and Technological Innovation Center Hangzhou 311215 China

5. State Key Laboratory of Silicon Materials and School of Materials Science and Engineering Zhejiang University Hangzhou 310027 China

Abstract

AbstractThe development of electric vehicles has received worldwide attention in the background of reducing carbon emissions, wherein lithium‐ion batteries (LIBs) become the primary energy supply systems. However, commercial graphite‐based anodes in LIBs currently confront significant difficulty in enduring ultrahigh power input due to the slow Li+ transport rate and the low intercalation potential. This will, in turn, cause dramatic capacity decay and lithium plating. The 2D layered materials (2DLMs) recently emerge as new fast‐charging anodes and hold huge promise for resolving the problems owing to the synergistic effect of a lower Li+ diffusion barrier, a proper Li+ intercalation potential, and a higher theoretical specific capacity with using them. In this review, the background and fundamentals of fast‐charging for LIBs are first introduced. Then the research progress recently made for 2DLMs used for fast‐charging anodes are elaborated and discussed. Some emerging research directions in this field with a short outlook on future studies are further discussed.

Funder

National Natural Science Foundation of China

China Postdoctoral Science Foundation

Publisher

Wiley

Subject

Biomaterials,Biotechnology,General Materials Science,General Chemistry

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